高级检索

    豫北典型耕地区土壤重金属分布特征及风险评价

    Distribution characteristics and risk assessment of heavy metals in cultivated soil in typical areas of northern Henan Province

    • 摘要:
      研究目的 探讨豫北典型耕作区重金属分布特征、污染水平,评估重金属健康风险并对超标严重区重金属来源进行解析。
      研究方法 系统采集161件表层土壤样品,测定重金属Cu、Pb、Zn、Cr、Cd、As、Ni和Hg的含量,采用内梅罗综合污染指数法和地累积指数评估重金属污染程度;采用潜在生态风险指数法评估其风险,运用健康风险评估模型对研究区成人和儿童的健康风险进行评估;采用PMF模型对重点区域土壤中8种重金属进行溯源分析。
      研究结果 除As外7种重金属元素均值均超河南省土壤背景值,且Cd有80.75%点位超风险筛选值;污染评价表明研究区整体处于轻度污染范围,Cd贡献率显著高于其他7种重金属,其次为Hg和Pb;潜在生态风险评价表明研究区处于高生态风险程度,存在生态风险的元素主要为Cd和Hg,贡献率分别为71.69%和21.89%;健康风险评价表明部分点位对成人和儿童的致癌风险以及儿童非致癌风险存在一定的健康风险,且风险程度表现为儿童>成人,引起健康风险的元素主要为As、Cr和Pb,需引起重视;通过相关性分析和PMF模型发现重点区域8种重金属有3种来源:As以岩石风化的自然源为主;Cd主要来源于工业废水排放源;其他6种重金属以交通运输源和煤炭燃烧源为主。3种来源贡献率分别为8.27%、2.34%和89.39%。
      结论 研究区耕地土壤重金属污染区主要集中在凤泉区和牧野区,Cd为主要贡献因子。As、Cr和Pb是健康风险的主要贡献因子。

       

      Abstract:
      This paper is the result of environmental geological survey engineering.
      Objective This study explored the distribution characteristics, pollution levels, and health risks of heavy metals in typical farming areas in northern Henan Province, China, and analyzed the sources of heavy metals in heavily polluted areas.
      Methods A total of 161 surface soil samples were systematically collected, and the concentrations of heavy metals such as Cu, Pb, Zn, Cr, Cd, As, Ni, and Hg were determined. The Nemero Comprehensive Pollution Index and Geological Accumulation Index were used to assess the degree of heavy metal pollution. The potential ecological risk index method was used to assess the risk. The health risk assessment model was used to assess the health risks of adults and children in the study area. Using the PMF model to trace the sources of eight heavy metals in key area soil.
      Results Except for As, the mean values of 7 heavy metal elements all exceeded the soil background values in Henan Province,, and 80.75% of the stations exceeding risk screening values for Cd. The pollution assessment showed that the study area was generally in a mildly polluted range, with Cd contributing significantly more than the other seven heavy metals, followed by Hg and Pb. The potential ecological risk assessment showed that the study area was at a high ecological risk level, with Cd and Hg as the main contributors to ecological risks, accounting for 71.69% and 21.89% respectively. The health risk assessment showed that some stations had certain health risks for adults and children, including carcinogenic risks for children and non-carcinogenic risks for adults. The risk levels were shown to be higher for children than for adults, with As, Cr, and Pb being the main contributors to health risks. Through correlation analysis and PMF modeling, it was found that there were three sources of heavy metals in key areas: As mainly came from natural sources such as rock weathering; Cd mainly came from industrial wastewater discharge sources; and the other six heavy metals mainly came from transportation sources and coal combustion sources. The contribution rates of the three sources are 8.27%, 2.34%, and 89.39%.
      Conclusion The heavy metal pollution areas in cultivated soil in the study area were mainly concentrated in Fengquan District and Muye District, with Cd as the main contributor. As, Cr, and Pb were the main contributors to health risks.

       

    /

    返回文章
    返回