石家庄市大气降尘重金属元素来源分析
DOI:
作者:
作者单位:

作者简介:

通讯作者:

中图分类号:

基金项目:

中国地质调查局和河北省政府合作项目“河北省多目标地球化学调查” (200040007-2)资助。


An analysis of the sources of heavy metals in atmospheric dustfall of Shijiazhuang City
Author:
Affiliation:

Fund Project:

  • 摘要
  • |
  • 图/表
  • |
  • 访问统计
  • |
  • 参考文献
  • |
  • 相似文献
  • |
  • 引证文献
  • |
  • 资源附件
  • |
  • 文章评论
    摘要:

    提要:本文对石家庄市大气降尘重金属含量水平进行了研究,从2007年11月起连续收集一年的大气降尘样品,分析了As、Cd、Hg、Pb、Cr、Cu、Zn、Ni、Mo、Mn、Al2O3、K2O等12项。结果表明,与土壤背景值相比,石家庄市大气降尘中除Al2O3外的重金属含量总体明显升高。采用相关分析和主成分分析,对降尘重金属元素来源进行解析,认为有3种主要来源:一是Pb、Cr、As、Hg、Mo、Cd、Mn与燃煤活动、道路交通有关;二是Ni、Cu、Zn除与燃煤活动有关外,还与工矿企业废气排放有关;三是Al2O3主要与土壤颗粒物有关(自然来源)。以Al作为参考元素计算重金属的富集因子表明,受工业活动影响的Cd、Hg、Zn具有较大的富集因子,大气降尘中的重金属含量高值区与工业区域的分布相吻合。

    Abstract:

    Abstract:Fifty-one atmospheric dustfall samples were collected successively from November 2007 to November 2008 in Shijiazhuang. All dustfall samples were analyzed for concentrations of As, Cd, Hg, Pb, Cr, Cu, Zn, Ni, Mn, Mo, Al2O3 and K2O. The results indicate that, compared with the background values of soil in Shijiazhuang area, atmospheric dustfalls have elevated metal concentrations on the whole, except for the concentration of Al2O3. Correlation coefficient analysis and principal component analysis (PCA) were performed and three main sources were identified: (1) Pb, Cr, As, Hg, Mo, Cd and Mn, which are mainly derived from coal combustion and traffic pollution; (2) Ni, Cu and Zn, which are probably related not only to coal combustion but also to factory exhaust; (3) Al2O3, which is mainly derived from soil particles. Based on concentration analysis and correlation analysis, the authors selected Al as the reference element to calculate the heavy metal enrichment factors (EFs), which in turn further validated the source identification. However, industrally enhanced Cd, Hg and Zn show maximum enrichments. Therefore, EFs shed a light on the level of human influence on atmospheric dustfalls. High concentrations of heavy metals in atmospheric dustfalls are consistent with the distribution of the industrial area.

    参考文献
    相似文献
    引证文献
引用本文

崔邢涛 栾文楼 李随民 宋泽峰. 石家庄市大气降尘重金属元素来源分析[J]. 中国地质, 2012, 39(4): 1108-1115.
CUI Xing-tao, LUAN Wen-lou, LI Sui-min, SONG Ze-feng. An analysis of the sources of heavy metals in atmospheric dustfall of Shijiazhuang City[J]. Geology in China, 2012, 39(4): 1108-1115(in Chinese with English abstract).

复制
分享
文章指标
  • 点击次数:
  • 下载次数:
  • HTML阅读次数:
  • 引用次数:
历史
  • 收稿日期:
  • 最后修改日期:
  • 录用日期:
  • 在线发布日期: 2012-11-08
  • 出版日期:
亮点文章推荐
古人云:工欲善其事,必先利其器。我国新一轮战略找矿行动已全面启动。用什么方法、什么手段实现增储上产是面临的突出问题。本刊登载了几篇基于新技术、新方法实现找矿突破的实例,供大家参阅,助力新一轮战略找矿目标的实现。
基于随机森林算法的找矿预测——以冈底斯成矿带西段斑岩—浅成低温热液型铜多金属矿为例. 欧阳渊等,2023, 50(2):303-330.
基于重磁资料在山东齐河—禹城探获矽卡岩型富铁矿:对超深覆盖区找矿的启示. 王润生等,2023, 50(2):331-346.
自然伽马曲线重构波阻抗反演在勘探含铀有利成矿砂体中的尝试. 梁建刚等,2023, 50(2):347-358.
宽频大地电磁法寻找“界面型”隐伏金矿床:以黔西南戈塘地区深部找矿为例. 张伟等,2023, 50(2):359-375.
页岩气基础地质调查钻井技术研究进展及展望. 赵洪波等,2023, 50(2):376-394.
关闭